Watched the video - my points stand. This is an interesting experiment but not much more, at least not on that particular mobo. There's even a CACHECHK result posted at 21m:15s and it's pretty obvious the mobo is only caching the first 32MiB. Still OKish to use as a RAMdisk (if it can be installed using top of memory) but not really otherwise. In fact an OS that's capable of using all that memory (like Win9x or Linux) might throw in some frequently accessed code or data there and now you have a system that's slower than 32M one.
OPTi 82C495SLC is not a great 386 chipset. It's not bad as such, and it's stable, but the RAM timings are pretty bad compared to something like Unichip U4800-VLX. So the fact these these are newer, 50ns chips doesn't matter here. Also the bank interleaving on OPTi is not really providing much of a boost but I would still prefer 16+16 configuration.
I have one criticism of this project though, and that is the use of 3V3 chips in 5V system. It's not enough to provide the correct supply voltage - the I/O levels must also be matched. These are LVTTL chips and not 5V tolerant, although the datasheet states that the upper limit is 4.6V - that's high enough that these won't die soon. But the overshoots during swithing, and possibly chipset write levels, will degrage and damage the I/Os eventually.